Abstract
We study a model for photovoltaic energy collection consisting of a Mott-insulating layer in presence of acoustic phonons, coupled to two wide-band fermion leads at different chemical potentials and driven into a nonequilibrium steady state by a periodic electric field. We treat electron correlations with nonequilibrium dynamical mean-field theory using the so-called auxiliary master-equation approach as impurity solver and include dissipation by acoustic phonons via the Migdal approximation. For a small hybridization to the leads, we obtain a peak in the photocurrent as a function of the driving frequency which can be associated with impact ionization processes. For larger hybridizations the shallow peak suggests a suppression of impact ionization with respect to direct photovoltaic excitations. Acoustic phonons slightly enhance the photocurrent for small driving frequencies and suppress it at frequencies around the main peak at all considered hybridization strengths.
Original language | English |
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Article number | 195140 |
Journal | Physical Review B |
Volume | 106 |
Issue number | 19 |
DOIs | |
Publication status | Published - 15 Nov 2022 |
ASJC Scopus subject areas
- Electronic, Optical and Magnetic Materials
- Condensed Matter Physics